<?xml version="1.0" encoding="UTF-8"?>
<!DOCTYPE article PUBLIC "-//NLM//DTD Journal Publishing DTD v3.0 20080202//EN" "http://dtd.nlm.nih.gov/publishing/3.0/journalpublishing3.dtd">
<article xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink" article-type="research-article" dtd-version="3.0" xml:lang="en">
<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACP</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7324</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>GÃ¶ttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acp-11-1339-2011</article-id>
<title-group>
<article-title>Production, growth and properties of ultrafine atmospheric aerosol particles in an urban environment</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Salma</surname>
<given-names>I.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>BorsÃ³s</surname>
<given-names>T.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Weidinger</surname>
<given-names>T.</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Aalto</surname>
<given-names>P.</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Hussein</surname>
<given-names>T.</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Dal Maso</surname>
<given-names>M.</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Kulmala</surname>
<given-names>M.</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Institute of Chemistry, EÃ¶tvÃ¶s University, Budapest, Hungary</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>Department of Meteorology, EÃ¶tvÃ¶s University, Budapest, Hungary</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>Department of Physical Sciences, University of Helsinki, Finland</addr-line>
</aff>
<pub-date pub-type="epub">
<day>15</day>
<month>02</month>
<year>2011</year>
</pub-date>
<volume>11</volume>
<issue>3</issue>
<fpage>1339</fpage>
<lpage>1353</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
<self-uri xlink:href="http://www.atmos-chem-phys.net/11/1339/2011/acp-11-1339-2011.html">This article is available from http://www.atmos-chem-phys.net/11/1339/2011/acp-11-1339-2011.html</self-uri>
<self-uri xlink:href="http://www.atmos-chem-phys.net/11/1339/2011/acp-11-1339-2011.pdf">The full text article is available as a PDF file from http://www.atmos-chem-phys.net/11/1339/2011/acp-11-1339-2011.pdf</self-uri>
<abstract>
<p>Number concentrations of atmospheric aerosol particles were measured by a
flow-switching type differential mobility particle sizer in an electrical
mobility diameter range of 6â€“1000 nm in 30 channels near central Budapest
with a time resolution of 10 min continuously from 3 November 2008 to 2
November 2009. Daily median number concentrations of particles varied from
3.8 &amp;times; 10&lt;sup&gt;3&lt;/sup&gt; to 29 &amp;times;10&lt;sup&gt;3&lt;/sup&gt; cm&lt;sup&gt;âˆ’3&lt;/sup&gt; with a yearly median
of 11.8 &amp;times; 10&lt;sup&gt;3&lt;/sup&gt; cm&lt;sup&gt;âˆ’3&lt;/sup&gt;. Contribution of ultrafine particles to
the total particle number ranged from 58 to 92% with a mean ratio and
standard deviation of (79 &amp;plusmn;  6)%. Typical diurnal variation of the
particle number concentration was related to the major emission patterns in
cities, new particle formation, sinks of particles and meteorology. Shapes
of the monthly mean number size distributions were similar to each other.
Overall mean for the number median mobility diameter of the Aitken and
accumulation modes were 26 and 93 nm, respectively, which are substantially
smaller than for rural or background environments. The Aitken and
accumulation modes contributed similarly to the total particle number
concentrations at the actual measurement location. New particle formation
and growth unambiguously occurred on 83 days, which represent 27% of all
relevant days. Hence, new particle formation and growth are not rare
phenomena in Budapest. Their frequency showed an apparent seasonal variation
with a minimum of 7.3% in winter and a maximum of 44% in spring. New
particle formation events were linked to increased gas-phase H&lt;sub&gt;2&lt;/sub&gt;SO&lt;sub&gt;4&lt;/sub&gt;
concentrations. In the studied area, new particle formation is mainly
affected by condensation sink and solar radiation. The formation process
seems to be not sensitive to SO&lt;sub&gt;2&lt;/sub&gt;, which was present in a yearly median
concentration of 6.7 Î¼g m&lt;sup&gt;âˆ’3&lt;/sup&gt;. This suggests that the precursor gas
was always available in excess. Formation rate of particles with a diameter
of 6 nm varied between 1.65 and 12.5 cm&lt;sup&gt;âˆ’3&lt;/sup&gt; s&lt;sup&gt;âˆ’1&lt;/sup&gt; with a mean and
standard deviation of (4.2 &amp;plusmn; 2.5) cm&lt;sup&gt;âˆ’3&lt;/sup&gt; s&lt;sup&gt;âˆ’1&lt;/sup&gt;. Seasonal dependency
for the formation rate could not be identified. Growth curves of nucleated
particles were usually superimposed on the characteristic diurnal pattern of
road traffic direct emissions. The growth rate of the nucleation mode with a
median diameter of 6 nm varied from 2.0 to 13.3 nm h&lt;sup&gt;âˆ’1&lt;/sup&gt; with a mean and
standard deviation of (7.7 &amp;plusmn; 2.4) nm h&lt;sup&gt;âˆ’1&lt;/sup&gt;. There was an indicative
tendency for larger growth rates in summer and for smaller values in winter.
New particle formation events increased the total number concentration by a
mean factor and standard deviation of 2.3 &amp;plusmn; 1.1 relative to the
concentration that occurred immediately before the event. Several indirect
evidences suggest that the new particle formation events occurred at least
over the whole city, and were of regional type. The results and conclusions
presented are the first information of this kind for the region over
one-year long time period.</p>
</abstract>
<counts><page-count count="15"/></counts>
</article-meta>
</front>
<body/>
<back>
<ref-list>
<title>References</title>
<ref id="ref1">
<label>1</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Aalto, P., HÃ¤meri, K., Becker, E., Weber, R., Salm, J., MÃ¤kelÃ¤, J., Hoell, C., O&apos;Dowd, C., Karlsson, H., VÃ¤kevÃ¤, M., Koponen, I. K., Buzorius, G., and Kulmala, M.: Physical characterization of aerosol particles during nucleation events, Tellus, 53B, 344â€“358, 2001. </mixed-citation>
</ref>
<ref id="ref2">
<label>2</label><mixed-citation publication-type="other" xlink:type="simple"> Alam, A., Shi, J. P., and Harrison, R. M.: Observations of new particle formation in urban air, J. Geophys. Res., 108(D3), 4093, http://dx.doi.org/10.1029/2001JD001417doi:10.1029/2001JD001417, 2003. </mixed-citation>
</ref>
<ref id="ref3">
<label>3</label><mixed-citation publication-type="other" xlink:type="simple"> Andreae, M. O. and Rosenfeld, D.: Aerosolâ€“cloudâ€“precipitation interactions. Part 1. The nature and sources of cloud-active aerosols, Earth-Sci. Rev., 89, 13â€“41, 2008. </mixed-citation>
</ref>
<ref id="ref4">
<label>4</label><mixed-citation publication-type="other" xlink:type="simple"> Birmili, W., Berresheim, H., Plass-DÃ¼lmer, C., Elste, T., Gilge, S., Wiedensohler, A., and Uhrner, U.: The Hohenpeissenberg aerosol formation experiment (HAFEX): a long-term study including size-resolved aerosol, H&lt;sub&gt;2&lt;/sub&gt;SO&lt;sub&gt;4&lt;/sub&gt;, OH, and monoterpenes measurements, Atmos. Chem. Phys., 3, 361â€“376, http://dx.doi.org/10.5194/acp-3-361-2003doi:10.5194/acp-3-361-2003, 2003. </mixed-citation>
</ref>
<ref id="ref5">
<label>5</label><mixed-citation publication-type="other" xlink:type="simple"> Charron, A. and Harrison, R. M.: Primary particle formation from vehicle emissions during exhaust dilution in the roadside atmosphere, Atmos. Environ., 37, 4109â€“4119, 2003. </mixed-citation>
</ref>
<ref id="ref6">
<label>6</label><mixed-citation publication-type="other" xlink:type="simple"> Dal Maso, M., Kulmala, M., Lehtinen, K. E. J., MÃ¤kelÃ¤, J. M., and Aalto, P. P., and O&apos;Dowd, C.: Condensation and coagulation sinks and formation of nucleation mode particles in coastal and boreal forest boundary layers, J. Geophys. Res., 107(19D), 8097, http://dx.doi.org/10.1029/2001jd001053doi:10.1029/2001jd001053, 2002. </mixed-citation>
</ref>
<ref id="ref7">
<label>7</label><mixed-citation publication-type="other" xlink:type="simple"> Dal Maso, M., Kulmala, M., Riipinen, I., Wagner, R., Hussein, T., Aalto, P. P., and Lehtinen, K. E. J.: Formation and growth of fresh atmospheric aerosols: eight years of aerosol size distribution data from SMEAR II, HyytiÃ¤lÃ¤, Finland, Boreal Environ. Res., 10, 323â€“336, 2005. </mixed-citation>
</ref>
<ref id="ref8">
<label>8</label><mixed-citation publication-type="other" xlink:type="simple"> Dal Maso, M., HyvÃ¤rinen, A., Komppula, M., Tunved, P., Kerminen, V.-M., Lihavainen, H., Viisanen, Y., Hansson, H.-C., and Kulmala, M.: Annual and interannual variation in boreal forest aerosol particle number and volume concentration and their connection to particle formation, Tellus, B60, 495â€“508, http://dx.doi.org/10.1111/j.1600-0889.2008.00366.xdoi:10.1111/j.1600-0889.2008.00366.x, 2008. </mixed-citation>
</ref>
<ref id="ref9">
<label>9</label><mixed-citation publication-type="other" xlink:type="simple"> Hamed, A., Birmili, W., Joutsensaari, J., Mikkonen, S., Asmi, A., Wehner, B., Spindler, G., Jaatinen, A., Wiedensohler, A., Korhonen, H., Lehtinen, K. E. J., and Laaksonen, A.: Changes in the production rate of secondary aerosol particles in Central Europe in view of decreasing SO&lt;sub&gt;2&lt;/sub&gt; emissions between 1996 and 2006, Atmos. Chem. Phys., 10, 1071â€“1091, http://dx.doi.org/10.5194/acp-10-1071-2010doi:10.5194/acp-10-1071-2010, 2010. </mixed-citation>
</ref>
<ref id="ref10">
<label>10</label><mixed-citation publication-type="other" xlink:type="simple"> Hinds, W. C.: Aerosol technology: properties, behavior, and measurement of airborne particles, 2nd ed., Wiley-Interscience, New York, 1999. </mixed-citation>
</ref>
<ref id="ref11">
<label>11</label><mixed-citation publication-type="other" xlink:type="simple"> Holmes, N. S.: A review of particle formation events and growth in the atmosphere in the various environments and discussion of mechanistic implications, Atmos. Environ., 41, 2183â€“2201, 2007. </mixed-citation>
</ref>
<ref id="ref12">
<label>12</label><mixed-citation publication-type="other" xlink:type="simple"> Hussein, T., Dal Maso, M., PetÃ¤jÃ¤, T., Koponen, I. K., Paatero, P., Aalto, P. P., HÃ¤meri, K., and Kulmala, M.: Evaluation of an automatic algorithm for fitting the particle number size distributions, Boreal Env. Res., 10, 337â€“355, 2005. </mixed-citation>
</ref>
<ref id="ref13">
<label>13</label><mixed-citation publication-type="other" xlink:type="simple"> Jeong, C.-H., Hopke, P. K., Chalupa, D., and Utell, M.: Characteristics of nucleation and growth events of ultrafine particles measured in Rochester, NY, Environ. Sci. Technol., 38, 1933â€“1940, 2004. </mixed-citation>
</ref>
<ref id="ref14">
<label>14</label><mixed-citation publication-type="other" xlink:type="simple"> Jeong, C.-H., Evans, G. J., Hopke, P. K., Chalupa, D., and Utell, M. J.: Influence of atmospheric dispersion and new particle formation events on ambient particle number concentration in Rochester, United States, and Toronto, Canada, J. Air Waste Manage. Assoc., 56, 431â€“443, 2006. </mixed-citation>
</ref>
<ref id="ref15">
<label>15</label><mixed-citation publication-type="other" xlink:type="simple"> Kiendler-Scharr, A., Wildt, J., Dal Maso, M., Hohaus, T., Kleist, E., Mentel, T. F., Tillmann, R., Uerlings, R., Schurr, U., and Wahner, A.: New particle formation in forests inhibited by isoprene emissions, Nature, 461, 381â€“384, 2009. </mixed-citation>
</ref>
<ref id="ref16">
<label>16</label><mixed-citation publication-type="other" xlink:type="simple"> Kulmala, M. and Kerminen, V.-M.: On the growth of atmospheric nanoparticles, Atmos. Res., 90, 132â€“150, 2008. </mixed-citation>
</ref>
<ref id="ref17">
<label>17</label><mixed-citation publication-type="other" xlink:type="simple"> Kulmala, M., Pirjola, L., and MÃ¤kelÃ¤, J. M.: Stable sulphate clusters as a source of new atmospheric particles, Nature, 404, 66â€“69, 2000. </mixed-citation>
</ref>
<ref id="ref18">
<label>18</label><mixed-citation publication-type="other" xlink:type="simple"> Kulmala, M., Dal Maso, M., MÃ¤kelÃ¤, J. M., Pirjola, L., VÃ¤kevÃ¤, M., Aalto, P., Miikkulainen, P., HÃ¤meri, K., and O&apos;Dowd, C. D.: On the formation, growth and composition of nucleation mode particles, Tellus, B53, 479â€“490, 2001. </mixed-citation>
</ref>
<ref id="ref19">
<label>19</label><mixed-citation publication-type="other" xlink:type="simple"> Kulmala, M., VehkamÃ¤ki, H., PetÃ¤jÃ¤, T., Dal Maso, M., Lauri, A., Kerminen, V.-M., Birmili, W., and McMurry, P.: Formation and growth rates of ultrafine atmospheric particles: a review of observations, J. Aerosol Sci., 35, 143â€“176, 2004a. </mixed-citation>
</ref>
<ref id="ref20">
<label>20</label><mixed-citation publication-type="other" xlink:type="simple"> Kulmala, M., Laakso, L., Lehtinen, K. E. J., Riipinen, I., Dal Maso, M., Anttila, T., Kerminen, V.-M., HÃµrrak, U., Vana, M., and Tammet, H.: Initial steps of aerosol growth, Atmos. Chem. Phys., 4, 2553â€“2560, http://dx.doi.org/10.5194/acp-4-2553-2004doi:10.5194/acp-4-2553-2004, 2004b. </mixed-citation>
</ref>
<ref id="ref21">
<label>21</label><mixed-citation publication-type="other" xlink:type="simple"> Kulmala, M., PetÃ¤jÃ¤, T., MÃ¶nkkÃ¶nen, P., Koponen, I. K., Dal Maso, M., Aalto, P. P., Lehtinen, K. E. J., and Kerminen, V.-M.: On the growth of nucleation mode particles: source rates of condensable vapor in polluted and clean environments, Atmos. Chem. Phys., 5, 409â€“416, http://dx.doi.org/10.5194/acp-5-409-2005doi:10.5194/acp-5-409-2005, 2005a. </mixed-citation>
</ref>
<ref id="ref22">
<label>22</label><mixed-citation publication-type="other" xlink:type="simple"> Kulmala, M., Lehtinen, K. E. J., Laakso, L., Mordas, G., and HÃ¤meri, K.: On the existence of neutral atmospheric clusters, Boreal Env. Res., 10, 79â€“87, 2005b. </mixed-citation>
</ref>
<ref id="ref23">
<label>23</label><mixed-citation publication-type="other" xlink:type="simple"> Kulmala, M., Riipinen, I., SipilÃ¤, M., Manninen, H., PetÃ¤jÃ¤, T., Junninen, H., Dal Maso, M., Mordas, G., Mirme, A., Vana, M., Hirsikko, A., Laakso, L., Harrison, R. M., Hanson, I., Leung, C., Lehtinen, K. E. J., and Kerminen, V.-M.: Towards direct measurement of atmospheric nucleation, Science, 318, 89â€“92, 2007.  </mixed-citation>
</ref>
<ref id="ref24">
<label>24</label><mixed-citation publication-type="other" xlink:type="simple"> Lehtinen, K. E. J., Dal Maso, M., Kulmala, M., and Kerminen, V.-M.: Estimating nucleation rates from apparent particle formation rates and vice versa: Revised formulation of the Kerminen-Kulmala equation, J. Aerosol Sci. 38, 988â€“994, 2007. </mixed-citation>
</ref>
<ref id="ref25">
<label>25</label><mixed-citation publication-type="other" xlink:type="simple"> Maenhaut, W., Raes, N., Chi, X., Cafmeyer, J., Wang, W., and Salma, I.: Chemical composition and mass closure for fine and coarse aerosols at a kerbside in Budapest, Hungary, in spring 2002, X-ray Spectrom., 34, 290â€“296, 2005. </mixed-citation>
</ref>
<ref id="ref26">
<label>26</label><mixed-citation publication-type="other" xlink:type="simple"> Maricq, M. M., Podsiadlik, D. H., and Chase, R.: Examination of the size-resolved and transient nature of motor vehicle particle emissions, Environ. Sci. Technol., 33, 1618â€“1626, 1999. </mixed-citation>
</ref>
<ref id="ref27">
<label>27</label><mixed-citation publication-type="other" xlink:type="simple"> Metzger, A., Verheggen, B., Dommen, J., Duplissy, J., Prevot, A. S. H., Weingartner, E., Riipinen, I., Kulmala, M., Spracklen, D. V., Carslaw, K. S., and Baltensperger, U.: Evidence for the role of organics in aerosol particle formation under atmospheric conditions, P. Natl. Acad. Sci. USA, 107, 6646â€“6651, 2010. </mixed-citation>
</ref>
<ref id="ref28">
<label>28</label><mixed-citation publication-type="other" xlink:type="simple"> Mirme, S., Mirme, A., Minikin, A., Petzold, A., HÃµrrak, U., Kerminen, V.-M., and Kulmala, M.: Atmospheric sub-3 nm particles at high altitudes, Atmos. Chem. Phys., 10, 437â€“451, http://dx.doi.org/10.5194/acp-10-437-2010doi:10.5194/acp-10-437-2010, 2010. </mixed-citation>
</ref>
<ref id="ref29">
<label>29</label><mixed-citation publication-type="other" xlink:type="simple"> Morawska, L., Thomas, S., Bofinger, N., Wainwright, D., and Neale, D.: Comprehensive characterization of aerosols in a subtropical urban atmosphere: particle size distribution and correlation with gaseous pollutants, Atmos. Environ., 32, 2467â€“2478, 1998. </mixed-citation>
</ref>
<ref id="ref30">
<label>30</label><mixed-citation publication-type="other" xlink:type="simple"> Morawska, L., Ristovski, Z., Jayaratne, E. R., Keogh, D. U., and Ling, X.: Ambient nano and ultrafine particles from motor vehicle emissions: Characteristics, ambient processing and implications on human exposure, Atmos. Environ., 42, 8113â€“8138, 2008. </mixed-citation>
</ref>
<ref id="ref31">
<label>31</label><mixed-citation publication-type="other" xlink:type="simple"> OberdÃ¶rster, G., OberdÃ¶rster, E., and OberdÃ¶rster, J.: Nanotoxicology: an emerging discipline evolving from studies of ultrafine particles, Environ. Health Perspect., 113, 823â€“839, 2005. </mixed-citation>
</ref>
<ref id="ref32">
<label>32</label><mixed-citation publication-type="other" xlink:type="simple"> O&apos;Dowd, C., Aalto, P., HÃ¤meri, K., Kulmala, M., and Hoffmann, T.: Atmospheric particles from organic vapours, Nature, 416, 497â€“498, 2002. </mixed-citation>
</ref>
<ref id="ref33">
<label>33</label><mixed-citation publication-type="other" xlink:type="simple"> OKJ (National register of road vehicles, in Hungarian), Ministry of National Development, Budapest, 2010. </mixed-citation>
</ref>
<ref id="ref34">
<label>34</label><mixed-citation publication-type="other" xlink:type="simple"> Park, K., Park, J. Y., Kwak, J.-H., Cho, G. N., and Kim, J.-S.: Seasonal and diurnal variations of ultrafine particle concentration in urban Gwangju, Korea: Observation of ultrafine particle events, Atmos. Environ., 42, 788â€“799, 2008. </mixed-citation>
</ref>
<ref id="ref35">
<label>35</label><mixed-citation publication-type="other" xlink:type="simple"> PetÃ¤jÃ¤, T., Mauldin, III, R. L., Kosciuch, E., McGrath, J., Nieminen, T., Paasonen, P., Boy, M., Adamov, A., Kotiaho, T., and Kulmala, M.: Sulfuric acid and OH concentrations in a boreal forest site, Atmos. Chem. Phys., 9, 7435â€“7448, http://dx.doi.org/10.5194/acp-9-7435-2009doi:10.5194/acp-9-7435-2009, 2009. </mixed-citation>
</ref>
<ref id="ref36">
<label>36</label><mixed-citation publication-type="other" xlink:type="simple"> Qian, S., Sakurai, H., and McMurry, P. H.: Characteristics of regional nucleation events in urban East St. Louis, Atmos. Environ., 41, 4119â€“4127, 2007. </mixed-citation>
</ref>
<ref id="ref37">
<label>37</label><mixed-citation publication-type="other" xlink:type="simple"> Raes, F., Van Dingenen, R., Vignati, E., Wilson, J., Putard, J. P., Seinfeld, J. H., and Adams, P.: Formation and cycling of aerosols in the global troposphere, Atmos. Environ., 34, 4215â€“4240, 2000. </mixed-citation>
</ref>
<ref id="ref38">
<label>38</label><mixed-citation publication-type="other" xlink:type="simple"> Ristovski, Z., Morawska, L., Bofinger, N. D., and Hitchins, J.: Submicrometer and supermicrometer particulate emission from spark ignition vehicles, Environ. Sci. Technol., 32, 38â€“45,1998. </mixed-citation>
</ref>
<ref id="ref39">
<label>39</label><mixed-citation publication-type="other" xlink:type="simple"> Salma, I. and Maenhaut, W.: Changes in chemical composition and mass of atmospheric aerosol pollution between 1996 and 2002 in a Central European city, Environ. Pollut., 143, 479â€“488, 2006. </mixed-citation>
</ref>
<ref id="ref40">
<label>40</label><mixed-citation publication-type="other" xlink:type="simple"> Salma, I., Maenhaut, W., ZemplÃ©n-Papp, Ã‰., and ZÃ¡ray, Gy.: Comprehensive characterisation of atmospheric aerosols in Budapest: physicochemical properties of inorganic species, Atmos. Environ., 35, 4367â€“4378, 2001. </mixed-citation>
</ref>
<ref id="ref41">
<label>41</label><mixed-citation publication-type="other" xlink:type="simple"> Salma, I., Chi, X., and Maenhaut, W.: Elemental and organic carbon in urban canyon and background environments in Budapest, Hungary, Atmos. Environ., 38, 27â€“36, 2004. </mixed-citation>
</ref>
<ref id="ref42">
<label>42</label><mixed-citation publication-type="other" xlink:type="simple"> Salma, I., Ocskay, R., Raes, N., and Maenhaut, W.: Fine structure of mass size distributions in urban environment, Atmos. Environ., 39, 5363â€“5374, 2005.  </mixed-citation>
</ref>
<ref id="ref43">
<label>43</label><mixed-citation publication-type="other" xlink:type="simple"> Salma, I., Ocskay, R., Varga, I., and Maenhaut, W.: Surface tension of atmospheric humic-like substances in connection with relaxation, dilution, and solution pH, J. Geophys. Res., 111, D23205, http://dx.doi.org/10.1029/2005JD007015doi:10.1029/2005JD007015, 2006. </mixed-citation>
</ref>
<ref id="ref44">
<label>44</label><mixed-citation publication-type="other" xlink:type="simple"> Salma, I., Ocskay, R., Chi, X., and Maenhaut, W.: Sampling artefacts, concentrations and chemical composition of fine water-soluble organic carbon and humic-like substances in a continental urban atmospheric environment, Atmos. Environ., 41, 4106â€“4118, 2007. </mixed-citation>
</ref>
<ref id="ref45">
<label>45</label><mixed-citation publication-type="other" xlink:type="simple"> Seinfeld, J. H. and Pandis, S. N.: Atmospheric chemistry and physics, From air pollution to climate change, Wiley, New York, 1998. </mixed-citation>
</ref>
<ref id="ref46">
<label>46</label><mixed-citation publication-type="other" xlink:type="simple"> Shi, J. P. and Harrison, R. M.: Investigation of ultrafine particle formation during diesel exhaust dilution, Environ. Sci. Technol., 33, 3730â€“3736, 1999. </mixed-citation>
</ref>
<ref id="ref47">
<label>47</label><mixed-citation publication-type="other" xlink:type="simple"> SipilÃ¤, M., Lehtipalo, K., Kulmala, M., PetÃ¤jÃ¤, T., Junninen, H., Aalto, P. P., Manninen, H. E., KyrÃ¶, E.-M., Asmi, E., Riipinen, I., Curtius, J., Kürten, A., Borrmann, S., and O&apos;Dowd, C. D.: Applicability of condensation particle counters to measure atmospheric clusters, Atmos. Chem. Phys., 8, 4049â€“4060, http://dx.doi.org/10.5194/acp-8-4049-2008doi:10.5194/acp-8-4049-2008, 2008. </mixed-citation>
</ref>
<ref id="ref48">
<label>48</label><mixed-citation publication-type="other" xlink:type="simple"> SipilÃ¤, M., Berndt, T., PetÃ¤jÃ¤, T., Brus, T., Vanhanen, J., Stratmann, F., Patokoski, J., Mauldin III, R. L., HyvÃ¤rinen, A.-P., Lihavainen, H., and Kulmala, M.: The role of sulphuric acid in atmospheric nucleation, Science, 327, 1243â€“1246, 2010. </mixed-citation>
</ref>
<ref id="ref49">
<label>49</label><mixed-citation publication-type="other" xlink:type="simple"> Stolzenburg, M. R., McMurry, P. H., Sakurai, H., Smith, J. N., Mauldin III, R. L., Eisele, F. L., and Clement, C. F.: Growth rates of freshly nucleated atmospheric particles in Atlanta, J. Geophys. Res., 110, D22S05, http://dx.doi.org/10.1029/2005JD005935doi:10.1029/2005JD005935, 2005. </mixed-citation>
</ref>
<ref id="ref50">
<label>50</label><mixed-citation publication-type="other" xlink:type="simple"> VÃ¤kevÃ¤, M., HÃ¤meri, K., Puhakka, T., Nilsson, E., Hohti, K., and MÃ¤kelÃ¤, J.: Effects of meteorological processes on aerosol particle size distribution in an urban background area, J. Geophys. Res., 105, 9807â€“9821, 2000.  </mixed-citation>
</ref>
<ref id="ref51">
<label>51</label><mixed-citation publication-type="other" xlink:type="simple"> Watson, J. G., Chow, J. C., Park, K., and Lowenthal, D. H.: Nanoparticle and ultrafine particle events at the Fresno supersite, J. Air Waste Manage. Assoc., 56, 417â€“430, 2006. </mixed-citation>
</ref>
<ref id="ref52">
<label>52</label><mixed-citation publication-type="other" xlink:type="simple"> Woo, K. S., Chen, D. R., Pui, D. Y. H., and McMurry, P. H.: Measurement of Atlanta aerosol size distributions: observations of ultrafine particle events, Aerosol Sci. Technol., 34, 75â€“87, 2001. </mixed-citation>
</ref>
<ref id="ref53">
<label>53</label><mixed-citation publication-type="other" xlink:type="simple"> WÃ¥hlin, P., Palmgren, F., and Van Dingrnen, R.: Experimental studies of ultrafine particles in streets and the relationship to traffic, Atmos. Environ., 35, 63â€“69, 2001. </mixed-citation>
</ref>
<ref id="ref54">
<label>54</label><mixed-citation publication-type="other" xlink:type="simple"> Yli-Juuti, T., Riipinen, I., Aalto, P. P., Nieminen, T., Maenhaut, W., Janssens, I. A., Claeys, M., Salma, I., Ocskay, R., Hoffer, A., Imre, K., and Kulmala, M.: Characteristics of new particle formation events and cluster ions at K-puszta, Hungary, Boreal Environ. Res., 14, 683â€“698, 2009. </mixed-citation>
</ref>
<ref id="ref55">
<label>55</label><mixed-citation publication-type="other" xlink:type="simple"> Zhang, Q., Stanier, C. O., Canagaratna, M. R., Jayne, J. T., Worsnop, D. R., Pandis, S. N., and Jimenez, J. L.: Insights into the chemistry of new particle formation and growth events in Pittsburgh based on aerosol mass spectrometry, Environ. Sci. Technol., 38, 4797â€“4809, 2004a. </mixed-citation>
</ref>
<ref id="ref56">
<label>56</label><mixed-citation publication-type="other" xlink:type="simple"> Zhang, R., Suh, I., Zhao, J., Zhang, D., Fortner, E. C., Tie, X., Molina, L. T., and Molina, M. J.: Atmospheric new particle formation enhanced by organic acids, Science, 304, 1487â€“1490, 2004b. </mixed-citation>
</ref>
</ref-list>
</back>
</article>