1NILU-Norwegian Institute for Air Research, Kjeller, Norway
2Meteorological Institute, Ludwig-Maximilians-University, Munich, Germany
3Division for Biomedical Physics, Innsbruck Medical University, Innsbruck, Austria
Received: 10 Aug 2010 – Discussion started: 01 Oct 2010
Abstract. Rotational Raman scattering in the Earth's atmosphere explains the filling-in of Fraunhofer lines in the solar spectrum. A new model including first-order rotational Raman scattering has been developed, based on a reimplementation of the versatile discrete ordinate radiative transfer (DISORT) solver in the C computer language. The solver is fully integrated in the freely available libRadtran radiative transfer package. A detailed description is given of the model including the spectral resolution and a spectral interpolation scheme that considerably speeds up the calculations. The model is used to demonstrate the effect of clouds on top and bottom of the atmosphere filling-in factors and differential optical depths. Cloud effects on vertical profiles of the filling-in factor are also presented. The spectral behaviour of the model is compared against measurements under thunderstorm and aerosol loaded conditions.
Revised: 23 Sep 2011 – Accepted: 10 Oct 2011 – Published: 21 Oct 2011
Kylling, A., Mayer, B., and Blumthaler, M.: Technical Note: A new discrete ordinate first-order rotational Raman scattering radiative transfer model – implementation and first results, Atmos. Chem. Phys., 11, 10471-10485, doi:10.5194/acp-11-10471-2011, 2011.