ACP Atmospheric Chemistry and Physics ACP 1680-7324 Copernicus GmbH Göttingen, Germany 10.5194/acp-11-10205-2011 The breakup of levitating water drops observed with a high speed camera Emersic C. 1 Connolly P. J. 1 School of Earth, Atmospheric and Environmental Sciences, University of Manchester, Manchester, UK 11 10 2011 11 19 10205 10218 This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited. This article is available from http://www.atmos-chem-phys.net/11/10205/2011/acp-11-10205-2011.html The full text article is available as a PDF file from http://www.atmos-chem-phys.net/11/10205/2011/acp-11-10205-2011.pdf

Collision-induced water drop breakup in a vertical wind tunnel was observed using a high speed camera for interactions between larger drop sizes (up to 7 mm diameter) than have previously been experimentally observed. Three distinct collisional breakup types were observed and the drop size distributions from each were analysed for comparison with predictions of fragment distributions from larger drops by two sets of established breakup parameterisations. The observations showed some similarities with both parameterisations but also some marked differences for the breakup types that could be compared, particularly for fragments 1 mm and smaller. Modifications to the parameterisations are suggested and examined. Presented is also currently the largest dataset of bag breakup distributions observed. Differences between this and other experimental research studies and modelling parameterisations, and the associated implications for interpreting results are discussed. Additionally, the stochastic coalescence and breakup equation was solved computationally using a breakup parameterisation, and the evolving drop-size distribution for a range of initial conditions was examined. Initial cloud liquid water content was found to have the greatest influence on the resulting distribution, whereas initial drop number was found to have relatively little influence. This may have implications when considering the effect of aerosol on cloud evolution, raindrop formation and resulting drop size distributions. Calculations presented show that, using an ideal initial cloud drop-size distribution, ~1–3% of the total fragments are contributed from collisional breakup between drops of 4 and 6 mm.

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