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<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACP</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7324</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acp-10-9819-2010</article-id>
<title-group>
<article-title>Direct and semi-direct impacts of absorbing biomass burning aerosol on the climate of southern Africa: a Geophysical Fluid Dynamics Laboratory GCM sensitivity study</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Randles</surname>
<given-names>C. A.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Ramaswamy</surname>
<given-names>V.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Atmospheric and Oceanic Sciences Program, Princeton University, Princeton, New Jersey, USA</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>NOAA Geophysical Fluid Dynamics Laboratory, Princeton, New Jersey, USA</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>now at: Goddard Earth Sciences and Technology Center, University of Maryland, Baltimore County and NASA GSFC Code 613.3, Greenbelt, Maryland, USA</addr-line>
</aff>
<pub-date pub-type="epub">
<day>19</day>
<month>10</month>
<year>2010</year>
</pub-date>
<volume>10</volume>
<issue>20</issue>
<fpage>9819</fpage>
<lpage>9831</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
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<abstract>
<p>Tropospheric aerosols emitted from biomass burning reduce solar radiation at
the surface and locally heat the atmosphere. Equilibrium simulations using an
atmospheric general circulation model (GFDL AGCM) indicate that strong
atmospheric absorption from these particles can cool the surface and increase
upward motion and low-level convergence over southern Africa during the dry
season. These changes increase sea level pressure over land in the biomass
burning region and spin-up the hydrologic cycle by increasing clouds,
atmospheric water vapor, and, to a lesser extent, precipitation. Cloud
increases serve to reinforce the surface radiative cooling tendency of the
aerosol. Conversely, if the climate over southern Africa were hypothetically
forced by high loadings of scattering aerosol, then the change in the
low-level circulation and increased subsidence would serve to decrease
clouds, precipitation, and atmospheric water vapor. Surface cooling
associated with scattering-only aerosols is mitigated by warming from cloud
decreases. The direct and semi-direct climate impacts of biomass burning
aerosol over southern Africa are sensitive to the total amount of aerosol
absorption and how clouds change in response to the aerosol-induced heating
of the atmosphere.</p>
</abstract>
<counts><page-count count="13"/></counts>
</article-meta>
</front>
<body/>
<back>
<ref-list>
<title>References</title>
<ref id="ref1">
<label>1</label><mixed-citation publication-type="other" xlink:type="simple"> Abel, S. J., Highwood, E. J., Haywood, J. M., and Stringer, M. A.: The direct radiative effect of biomass burning aerosols over southern Africa, Atmos. Chem. Phys., 5, 1999–2018, doi:10.5194/acp-5-1999-2005, 2005. </mixed-citation>
</ref>
<ref id="ref2">
<label>2</label><mixed-citation publication-type="other" xlink:type="simple"> </mixed-citation>
</ref>
<ref id="ref3">
<label>3</label><mixed-citation publication-type="other" xlink:type="simple"> Anderson, J., Balaji, V., Broccoli, A. J., et al.: The new GFDL global atmosphere and land model AM2-LM2: Evaluation with prescribed SST simulations, J. Climate, 17, 4641–4673, 2004. </mixed-citation>
</ref>
<ref id="ref4">
<label>4</label><mixed-citation publication-type="other" xlink:type="simple"> Brioude, J., Cooper, O. R., Feingold, G. Trainer, M., Freitas, S. R., Kowal, D. Ayers, J. K., Prins, E., Minnis, P., McKeen, S. A., Frost, G. J., and Hsie, E.-Y.: Effect of biomass burning on marine stratocumulus clouds off the California coast, Atmos. Chem. Phys., 9, 22, 8841–8856, doi:10.5194/acp-8-8841-2009, 2009. </mixed-citation>
</ref>
<ref id="ref5">
<label>5</label><mixed-citation publication-type="other" xlink:type="simple"> Chakraborty, A., Satheesh, S. K., Nanjundiah, R. S., and Srinivasan, J.: Impact of absorbing aerosols on the simulation of climate over the Indian region in an atmospheric general circulation model, Ann. Geophys., 22, 1421–1434, 2004. </mixed-citation>
</ref>
<ref id="ref6">
<label>6</label><mixed-citation publication-type="other" xlink:type="simple"> Ch\&apos;ylek, P. and Coakley, J. A.: Aerosols and Climate, Science, 183, 75–77, 1974 </mixed-citation>
</ref>
<ref id="ref7">
<label>7</label><mixed-citation publication-type="other" xlink:type="simple"> Delworth, T. L., Broccoli, A. J., Rosati, A., et al.: GFDL&apos;s CM2 global coupled climate models- Part 1: Formulation and simulation characteristics, J. Climate, 19(5), 643–674, 2006. </mixed-citation>
</ref>
<ref id="ref8">
<label>8</label><mixed-citation publication-type="other" xlink:type="simple"> Garstang, M., Tyson, P. D., Swap, R., Edwards, M., Kållbert, P., and Lindesay, J. A.: Horizontal and vertical transport of air over southern Africa, J. Geophys. Res., 101, 23721–23736, 1996. </mixed-citation>
</ref>
<ref id="ref9">
<label>9</label><mixed-citation publication-type="other" xlink:type="simple"> Ginoux, P., Horowitz, L. W., Ramaswamy, V., Geogdzhayev, I. V., Holben, B. N., Stenchikov, G., and Tie, X.: Evaluation of aerosol distribution and optical depth in the Geophysical Fluid Dynamics Laboratory coupled model CM2.1 for present climate, J. Geophys. Res., 111, D22210, doi:10.1029/2005JD006707, 2006. </mixed-citation>
</ref>
<ref id="ref10">
<label>10</label><mixed-citation publication-type="other" xlink:type="simple"> Hackert, E. C. and Hastenrath, S.: Mechanisms of Java rainfall anomalies, Mon. Weather Rev., 114, 745–757, 1986. </mixed-citation>
</ref>
<ref id="ref11">
<label>11</label><mixed-citation publication-type="other" xlink:type="simple"> Hansen, J., Sato, M., and Ruedy, R.: Radiative forcing and climate response, Journal of Geophysical Research, 102(D6), 6831–6864, 1997. </mixed-citation>
</ref>
<ref id="ref12">
<label>12</label><mixed-citation publication-type="other" xlink:type="simple"> Haywood, J. M. and Ramaswamy, V.: Global Sensitivity studies of the direct radiative forcing due to anthropogenic sulfate and black carbon aerosols, J. Geophys. Res., 103(D6), 6043–6058, 1998. </mixed-citation>
</ref>
<ref id="ref13">
<label>13</label><mixed-citation publication-type="other" xlink:type="simple"> Haywood, J. M., Ramaswamy, V., and Soden, B. J.: Tropospheric aerosol climate forcing in clear-sky satellite observations over the oceans, Science, 283, 5406, 1299–1303, 1999. </mixed-citation>
</ref>
<ref id="ref14">
<label>14</label><mixed-citation publication-type="other" xlink:type="simple"> Haywood, J. M., Osborne, S. R., Francis, P. N., Keil, A., Formenti, P., Andreae, M. O., and Kaye, P. H.: The mean physical and optical properties of regional haze dominated by biomass burning aerosol measured from the C-130 aircraft during SAFARI 2000, J. Geophys. Res., 108(D13), 8473, doi:10.1029/2002JD002226, 2003. </mixed-citation>
</ref>
<ref id="ref15">
<label>15</label><mixed-citation publication-type="other" xlink:type="simple"> Holben, B., Tanre, D., Smirnov, A., et al.: An emerging ground-based aerosol climatology: Aerosol optical depth from AERONET, J. Geophys. Res., 106(D11), 12067–12097, 2001. </mixed-citation>
</ref>
<ref id="ref16">
<label>16</label><mixed-citation publication-type="other" xlink:type="simple"> Horowitz, L.: Past, present, and future concentrations of tropospheric ozone and aerosols: Methodology, ozone evaluation, and sensitivity to aerosol wet removal, J. Geophys. Res., 111, D22211, doi:10.1029/2005JD006937, 2006. </mixed-citation>
</ref>
<ref id="ref17">
<label>17</label><mixed-citation publication-type="other" xlink:type="simple"> Johnson, B. T., Shine, K. P., and Forster, P. M.: The semi-direct aerosol effect: Impact of absorbing aerosols on marine stratocumulus, Q. J. Roy. Meterol. Soc., 130(599), 1407–1422, 2004. </mixed-citation>
</ref>
<ref id="ref18">
<label>18</label><mixed-citation publication-type="other" xlink:type="simple"> Kaufman, Y. J., Tanre, D., Remer, L., Vermonte, E., Chu, A., and Holben, B. N.: Remote sensing of tropospheric aerosol over the land using dark targets and dynamic aerosol models,J. Geophys. Res., 102, 17051–17067, 1997. </mixed-citation>
</ref>
<ref id="ref19">
<label>19</label><mixed-citation publication-type="other" xlink:type="simple"> Keil, A. and Haywood, J. M.: Solar radiative forcing by biomass burning aerosol particles during SAFARI 2000: A case study based on measured aerosol and cloud properties, J. Geophys. Res., 108(D13), 8467, doi:10.1029/2002JD002315, 2003. </mixed-citation>
</ref>
<ref id="ref20">
<label>20</label><mixed-citation publication-type="other" xlink:type="simple"> Koch, D. and Del Genio, A. D.: Black carbon semi-direct effects on cloud cover: review and synthesis, Atmos. Chem. Phys., 10, 7685–7696, doi:10.5194/acp-10-7685-2010, 2010. </mixed-citation>
</ref>
<ref id="ref21">
<label>21</label><mixed-citation publication-type="other" xlink:type="simple"> Koch, D., Schulz, M., Kinne, S., McNaughton, C., Spackman, J. R., Balkanski, Y., Bauer, S., Berntsen, T., Bond, T. C., Boucher, O., Chin, M., Clarke, A., De Luca, N., Dentener, F., Diehl, T., Dubovik, O., Easter, R., Fahey, D. W., Feichter, J., Fillmore, D., Freitag, S., Ghan, S., Ginoux, P., Gong, S., Horowitz, L., Iversen, T., Kirkevåg, A., Klimont, Z., Kondo, Y., Krol, M., Liu, X., Miller, R., Montanaro, V., Moteki, N., Myhre, G., Penner, J. E., Perlwitz, J., Pitari, G., Reddy, S., Sahu, L., Sakamoto, H., Schuster, G., Schwarz, J. P., Seland, Ø., Stier, P., Takegawa, N., Takemura, T., Textor,  C., van Aardenne, J. A., and Zhao, Y.: Evaluation of black carbon estimations  in global aerosol models, Atmos. Chem. Phys., 9, 9001–9026, doi:10.5194/acp-9-9001-2009, 2009. </mixed-citation>
</ref>
<ref id="ref22">
<label>22</label><mixed-citation publication-type="other" xlink:type="simple"> Koren, I., Kaufman, Y. J., Remer, L. A., and Martins, J. V.: Measurement of the effect of Amazon smoke on inhibation of cloud formation, Science, 303, 1342–1345, doi:10.1126/science.1089424, 2004. </mixed-citation>
</ref>
<ref id="ref23">
<label>23</label><mixed-citation publication-type="other" xlink:type="simple"> Koster, R. D., Suarez, M. J., Liu, P., et. al.: Regions of strong coupling between soil moisture and precipitation, Science, 305, 1138–1140, 2004. </mixed-citation>
</ref>
<ref id="ref24">
<label>24</label><mixed-citation publication-type="other" xlink:type="simple"> Lau, K. M., Kim, K. M., Sud, Y. C., and Walker, G. K.: A GCM study of the response of the atmospheric water cycle of West Africa an the Atlantic to Saharan dust radiative forcing, Ann. Geophys., 27, 4023–4037, doi:10.5194/angeo-27-4023-2009, 2009. </mixed-citation>
</ref>
<ref id="ref25">
<label>25</label><mixed-citation publication-type="other" xlink:type="simple"> Lau, K. M., Kim, M. K., and Kim, K. M.: Asian summer monsoon anomalies induced by aerosol direct forcing: The role of the Tibetan Plateau, Clim. Dynam., 26(7–8), 855–864, 2006. </mixed-citation>
</ref>
<ref id="ref26">
<label>26</label><mixed-citation publication-type="other" xlink:type="simple"> Leahy, L. V., Anderson, T. L., Eck, T. F., and Bergstrom, R. W.: A Synthesis of biomass burning aerosol over southern Africa during SAFARI 2000, Geophys. Res. Lett., 34, L12814, doi:10.1029/2007GL029697, 2007. </mixed-citation>
</ref>
<ref id="ref27">
<label>27</label><mixed-citation publication-type="other" xlink:type="simple"> Magi, B.: Chemical apportionment of southern African aerosol mass and optical depth, Atmos. Chem. Phys., 9, 7643–7655, doi:10.5194/acp-9-7643-2009, 2009. </mixed-citation>
</ref>
<ref id="ref28">
<label>28</label><mixed-citation publication-type="other" xlink:type="simple"> Magi, B. I., Ginoux, P., Ming, Y., and Ramaswamy, V.: Evaluation of tropical and extratropical Southern Hemisphere African aerosol properties simulated by a climate model, J. Geophys. Res., 114, D14204, doi:10.1029/2008JD011128, 2009. </mixed-citation>
</ref>
<ref id="ref29">
<label>29</label><mixed-citation publication-type="other" xlink:type="simple"> Magi, B. I. and Hobbs, P. V.: Hobbs: Effects of humidity on aerosols in southern Africa during the biomass burning season, J. Geophys. Res., 108(D13), 8495, doi:10.1029/2002JD002144, 2003. </mixed-citation>
</ref>
<ref id="ref30">
<label>30</label><mixed-citation publication-type="other" xlink:type="simple"> Menon, S., Hansen, J., Nazarenko, L., and Luo, Y.: Climate effects of black carbon aerosols in China and India, Science, 297, 2250–2253, 2002. </mixed-citation>
</ref>
<ref id="ref31">
<label>31</label><mixed-citation publication-type="other" xlink:type="simple"> Miller, R. L., Tegen, I., and Perlwitz, J.: Surface radiative forcing by soil dust aerosols and the hydrologic cycle, J. Geophys. Res., 109, D04203, doi:10.1029/2003JD004085, 2004. </mixed-citation>
</ref>
<ref id="ref32">
<label>32</label><mixed-citation publication-type="other" xlink:type="simple"> Ming, Y., Ramaswamy, V., Ginoux, P. A., and Horowitz, L. H.: Direct radiative forcing of anthropogenic organic aerosol, J. Geophys. Res., 110, D20208, doi:10.1029/2004JD005573, 2005. </mixed-citation>
</ref>
<ref id="ref33">
<label>33</label><mixed-citation publication-type="other" xlink:type="simple"> Myhre, G., Bernsten, T. K., Haywood, J. M., Sundet, J. K., Holben, B. N., Johnsrud, M., and Stordal, F.: Modeling the solar radiative impact of aerosols from biomass burning during the Southern African Regional Science Initiative (SAFARI-2000) experiment, J. Geophys. Res., 108(D13), 8501, doi:10.1029/2002JD002313, 2003. </mixed-citation>
</ref>
<ref id="ref34">
<label>34</label><mixed-citation publication-type="other" xlink:type="simple"> Ott, L., Duncan, B., Pawson, S., Colarco, P. R., Chin, M., Randles, C., Diehl, T., and Nielsen, E.: The influence of the 2006 Indonesian biomass burning aerosols on tropical dynamics studied with the GEOS-5 AGCM, J. Geophys. Res., doi:10.1029/2009JD013181, D14121, 2010. </mixed-citation>
</ref>
<ref id="ref35">
<label>35</label><mixed-citation publication-type="other" xlink:type="simple"> Paeth, H. and Feichter, J: Greenhouse-gas versus aerosol forcing and African climate response, Clim. Dynam., 26, 35–54, 2006. </mixed-citation>
</ref>
<ref id="ref36">
<label>36</label><mixed-citation publication-type="other" xlink:type="simple"> Ramanathan V. and Carmichael, G.: Global and regional climate changes due to black carbon, Nat. Geosci., 1, 221–227, 2008. </mixed-citation>
</ref>
<ref id="ref37">
<label>37</label><mixed-citation publication-type="other" xlink:type="simple"> Ramanathan, V., Chung, C., Kim, D., Bettge, T., Buja, L., Kiehl, J. T., Washington, W. M., Fu, Q., Sikka, D. R., and Wild, M.: Atmospheric brown clouds: Impacts on South Asian climate and hydrological cycle, P. Natl. Acad. Sci., 102, 15, 5326–5333, 2005. </mixed-citation>
</ref>
<ref id="ref38">
<label>38</label><mixed-citation publication-type="other" xlink:type="simple"> Randles, C. A. and Ramaswamy, V.: Absorbing aerosols over Asia: A GFDL general circulation model sensitivity study of model response to aerosol optical depth and aerosol absorption, J. Geophys. Res., 113, D21203, doi:10.1029/2008JD010140, 2008. </mixed-citation>
</ref>
<ref id="ref39">
<label>39</label><mixed-citation publication-type="other" xlink:type="simple"> Reynolds, R. W., Rayner, N. A., Smith, T. M., Stockes, D. C., and Wang, W.: An improved in situ and satellite SST analysis for climate, J. Climate, 15, 1609–1625, 2002. </mixed-citation>
</ref>
<ref id="ref40">
<label>40</label><mixed-citation publication-type="other" xlink:type="simple"> Roeckner, E., Stier, P., Feichter, J., Kloster, S., Esch, M., and Fischer-Bruns, L.: Impact of carbonaceous aerosol emissions on regional climate change, Clim. Dynam., 27, 552–571, 2006. </mixed-citation>
</ref>
<ref id="ref41">
<label>41</label><mixed-citation publication-type="other" xlink:type="simple"> Solomon S., Qin, D., Manning, M., et al.: Technical Summary Contribution of Working Group 1 to the 4th Assessment Report of the Intergovernmental Panel on Climate Change, in: Climate Change 2007: The Physical Science Basis, Cambridge University Press, New York, USA, 21–87, 2007. </mixed-citation>
</ref>
<ref id="ref42">
<label>42</label><mixed-citation publication-type="other" xlink:type="simple"> Swap, R. J., Annegarn, H. J., Suttles, J. T., King, M. D., Platnick, S., Privette, J. L., and Scholes, R. J.: Africa burning: A thematic analysis of the Southern African Regional Science Initiative (SAFARI 2000), J. Geophys. Res., 108(D13), 8465, doi:10.1029/2003JD003747, 2003. </mixed-citation>
</ref>
<ref id="ref43">
<label>43</label><mixed-citation publication-type="other" xlink:type="simple"> Torres, O., Bhartia, P. K., Herman, J. R., Ahmad, Z., and Gleason, J.: Derivation of aerosol properties from satellite measurements of backscattered ultraviolet radiation: Theoretical basis, J. Geophys. Res., 103, 17099–17110, 1998. </mixed-citation>
</ref>
<ref id="ref44">
<label>44</label><mixed-citation publication-type="other" xlink:type="simple"> Torres, O., Bhartia, P. K., Herman, J. R., Syniuk, A., Ginoux, P., and Holben, B.: A long-term record of aerosol optical depth from TOMS observations and comparison to AERONET measurements, J. Atmos. Science, 59, 398–413, 2002. </mixed-citation>
</ref>
<ref id="ref45">
<label>45</label><mixed-citation publication-type="other" xlink:type="simple"> Torres, O., Bhartia, P. K., Sinyuk, a., Welton, E. J., and Holben, B.: Total Ozone Mapping Spectrometer measurements of aerosol absorption from space: Comparison to SAFARI 2000 ground-based observations, J. Geophys. Res., 110, D10S18, doi:10.1029/2004JD004611, 2005. </mixed-citation>
</ref>
</ref-list>
</back>
</article>