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<article language="en">
	<journal>
		<journal_title>Atmospheric Chemistry and Physics</journal_title>
		<journal_url>www.atmos-chem-phys.net</journal_url>
		<issn>1680-7316</issn>
		<eissn>1680-7324</eissn>
		<volume_number>10</volume_number>
		<issue_number>1</issue_number>
		<publication_year>2010</publication_year>
	</journal>
	<doi>10.5194/acp-10-83-2010</doi>
	<article_url>http://www.atmos-chem-phys.net/10/83/2010/</article_url>
	<abstract_html>http://www.atmos-chem-phys.net/10/83/2010/acp-10-83-2010.html</abstract_html>
	<fulltext_pdf>http://www.atmos-chem-phys.net/10/83/2010/acp-10-83-2010.pdf</fulltext_pdf>
	<start_page>83</start_page>
	<end_page>94</end_page>
	<publication_date>2010-01-07</publication_date>
	<article_title content_type="html">High resolution modeling of CO&lt;sub&gt;2&lt;/sub&gt; over Europe: implications for representation errors of satellite retrievals</article_title>
	<authors>
		<author numeration="1" affiliations="1">
			<name>D. Pillai</name>
			<email>kdhanya@bgc-jena.mpg.de</email>
		</author>
		<author numeration="2" affiliations="1">
			<name>C. Gerbig</name>
		</author>
		<author numeration="3" affiliations="1">
			<name>J. Marshall</name>
		</author>
		<author numeration="4" affiliations="2,3">
			<name>R. Ahmadov</name>
		</author>
		<author numeration="5" affiliations="1">
			<name>R. Kretschmer</name>
		</author>
		<author numeration="6" affiliations="1">
			<name>T. Koch</name>
		</author>
		<author numeration="7" affiliations="1">
			<name>U. Karstens</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">Max Planck Institute for Biogeochemistry, P.O. Box 100164, 07701 Jena, Germany</affiliation>
		<affiliation numeration="2" content_type="html">NOAA Earth System Research Laboratory, Boulder, Colorado, USA</affiliation>
		<affiliation numeration="3" content_type="html">also at: Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, USA</affiliation>
	</affiliations>
	<abstract content_type="html">Satellite retrievals for column CO&lt;sub&gt;2&lt;/sub&gt; with better spatial and temporal
sampling are expected to improve the current surface flux estimates of
CO&lt;sub&gt;2&lt;/sub&gt; via inverse techniques. However, the spatial scale mismatch between
remotely sensed CO&lt;sub&gt;2&lt;/sub&gt; and current generation inverse models can induce
representation errors, which can cause systematic biases in flux estimates.
This study is focused on estimating these representation errors associated
with utilization of satellite measurements in global models with a
horizontal resolution of about 1 degree or less. For this we used simulated
CO&lt;sub&gt;2&lt;/sub&gt; from the high resolution modeling framework WRF-VPRM, which links
CO&lt;sub&gt;2&lt;/sub&gt; fluxes from a diagnostic biosphere model to a weather forecasting
model at 10&amp;times;10 km&lt;sup&gt;2&lt;/sup&gt; horizontal resolution. Sub-grid variability of
column averaged CO&lt;sub&gt;2&lt;/sub&gt;, i.e. the variability not resolved by global
models, reached up to 1.2 ppm with a median value of 0.4 ppm. Statistical
analysis of the simulation results indicate that orography plays an
important role. Using sub-grid variability of orography and CO&lt;sub&gt;2&lt;/sub&gt; fluxes
as well as resolved mixing ratio of CO&lt;sub&gt;2&lt;/sub&gt;, a linear model can be
formulated that could explain about 50% of the spatial patterns in the
systematic (bias or correlated error) component of representation error in
column and near-surface CO&lt;sub&gt;2&lt;/sub&gt; during day- and night-times. These findings
give hints for a parameterization of representation error which would allow
for the representation error to taken into account in inverse models or data
assimilation systems.</abstract>
	<references>
		<reference numeration="1" content_type="text"> Ahmadov, R., Gerbig, C., Kretschmer, R., Koerner, S., Neininger, B., Dolman, A. J., and Sarrat,C.: Mesoscale covariance of transport and CO2 fluxes: Evidence from observations and simulations using the WRF-VPRM coupled atmosphere-biosphere model, J. Geophys. Res.-Atmos., 112, D22107, doi:22110.21029/22007JD008552, 2007. </reference>
		<reference numeration="2" content_type="text"> Alkhaled, A. A., Michalak, A. M., and Kawa, S. R.: Using CO2 spatial variability to quantify representation errors of satellite CO2 retrievals, Geophys. Res. Lett., 35, L16813, doi:10.1029/2008GL034528, 2008. </reference>
		<reference numeration="3" content_type="text"> Chevillard, A., Karstens, U., Ciais, P., Lafont, S., and Heimann, M.: Simulation of atmospheric CO2 over Europe and western Siberia using the regional scale model REMO, Tellus B, 54B, 872–894, 2002. </reference>
		<reference numeration="4" content_type="text"> Corbin, K. D., Denning, A. S., Lu, L., Wang, J.-W., and Baker, I. T.: Possible representation errors in inversions of satellite CO2 retrievals, J. Geophys. Res.-Atmos., 113, D02301, doi:10.1029/2007JD008716, 2008. </reference>
		<reference numeration="5" content_type="text"> Crisp, D., Atlas, R. M., Breon, F.-M., Brown, L. R., Burrows, J. P., Ciais, P., Connor, B. J.,Doney, S. C., Fung, I. Y., Jacob, D. J., Miller, C. E., O&apos;Brien, D., Pawson, S., Randerson, J.T., Rayner, P., Salawitch, R. J., Sander, S. P., Sen, B., Stephens, G. L., Tans, P. P., Toon, G. C., Wennberg, P. O., Wofsy, S. C., Yung, Y. L., Kuang, Z., Chudasama, B., Sprague, G.,Weiss, B., Pollock, R., Kenyon, D., and Schroll, S.: The Orbiting Carbon Observatory (OCO) mission, Adv. Space Res., 34, 700–709, 2004. </reference>
		<reference numeration="6" content_type="text"> ESA: European Space Agency Mission Assessment Reports-ASCOPE, online available at: http://esamultimedia.esa.int/docs/SP1313-1_ASCOPE.pdf, 2008. </reference>
		<reference numeration="7" content_type="text"> Friedlingstein, P., Cox, P., Betts, R., Bopp, L., von Bloh, W., Brovkin, V., Cadule, P., Doney, S., Eby, M., Fung, I., Bala, G., John, J., Jones, C., Joos, F., Kato, T., Kawamiya, M., Knorr, W.,Lindsay, K., Matthews, H. D., Raddatz, T., Rayner, P., Reick, C., Roeckner, E., Schnitzler, K.-G., Schnur, R., Strassmann, K., Weaver, A. J., Yoshikawa, C., and Zeng, N.: Climate carbon cycle feedback analysis: Results from the C4MIP model intercomparison, J. Climate, 19, 3337–3353, 2006. </reference>
		<reference numeration="8" content_type="text"> Galmarini, S., Vinuesa, J.-F., and Martilli, A.: Modeling the impact of sub-grid scale emission variability on upper-air concentration, Atmos. Chem. Phys., 8, 141–158, 2008. </reference>
		<reference numeration="9" content_type="text"> Gerbig, C., Lin, J. C., Wofsy, S. C., Daube, B. C., Andrews, A. E., Stephens, B. B., Bakwin, P. S., and Grainger, C. A.: Toward constraining regional-scale fluxes of CO2 with atmospheric observations over a continent: 1. Observed spatial variability from airborne platforms, J. Geophys. Res.-Atmos., 108, 4756, doi:4710.1029/2002JD003018, 2003. </reference>
		<reference numeration="10" content_type="text"> Grell, G. A., Peckham, S. E., Schmitz, R., McKeen, S. A., Frost, G., Skamarock, W. C., and Eder, B.: Fully coupled online chemistry within the WRF model, Atmos. Environ., 39, 6957–6975, 2005. </reference>
		<reference numeration="11" content_type="text"> Gurney, K. R., Law, R. M., Denning, A. S., Rayner, P. J., Baker, D., Bousquet, P., Bruhwiler, L., Chen, Y.-H., Ciais, P., Fan, S. M., Fung, I. Y., Gloor, M., Heimann, M., Higuchi, K., John, J., Kowalczyk, E., Maki, T., Maksyutov, S., Peylin, 5 P., Prather, M., Pak, B. C., Sarmiento, J., Taguchi, S., Takahashi, T., and Yuen, C.-W.: TransCom 3 CO2 inversion intercomparison: 1. Annual mean control results and sensitivity to transport and prior flux information, Tellus B, 55, 555–579, 2003. </reference>
		<reference numeration="12" content_type="text"> Heimann, M., Koerner, S., Tegen, I., and Werner, M.: The global atmospheric tracer model TM3, Max-Planck Institut für Biogeochemie, Technical Reports 5, 131 pp., 2003. </reference>
		<reference numeration="13" content_type="text"> IPCC: Climate Change 2007: Synthesis Report. Contribution of Working Groups I, II and III to the Fourth Assessment Report of the Intergovernmental Panel on Climate Change, edited by: Core Writing Team, Pachauri, R. K., and Reisinger, A., IPCC, Cambridge University Press, Cambridge, 104 pp., 2007. </reference>
		<reference numeration="14" content_type="text"> Jung, M., Henkel, K., Herold, M., and Churkina, G.: Exploiting synergies of global land cover products for carbon cycle modeling, Remote Sens. Environ., 101, 534–553, 2006. </reference>
		<reference numeration="15" content_type="text"> Law, R. M., Peters, W., R\&quot; odenbeck, C., Aulagnier, C., Baker, I., Bergmann, D. J., Bousquet, P., Brandt, J., Bruhwiler, L., Cameron-Smith, P. J., Christensen, J. H., Delage, F., Denning, A. S., Fan, S., Geels, C., Houweling, S., Imasu, R., Karstens, U., Kawa, S. R., Kleist, J., Krol, M. C., Lin, S.-J., Lokupitiya, R., Maki, T., Maksyutov, S., Niwa, Y., Onishi, R., Parazoo, N., Patra, P. K., Pieterse, G., Rivier, L., Satoh, M., Serrar, S., Taguchi, S., Takigawa, M., Vautard, R., Vermeulen, A. T., and Zhu, Z.: TransCom model simulations of hourly atmospheric CO2: Experimental overview and diurnal cycle results for 2002, Global Biogeochem. Cy., 22, GB3009, doi:3010.1029/2007GB003050, 2008. </reference>
		<reference numeration="16" content_type="text"> Lin, J. C., Gerbig, C., Daube, B. C., Wofsy, S. C., Andrews, A. E., Vay, S. A., and Anderson, B. E.: An empirical analysis of the spatial variability of atmospheric CO2: Implications for inverse analyses and space-borne sensors, Geophys. Res. Lett., 31, L23104, doi:23110.21029/22004GL020957, 2004. </reference>
		<reference numeration="17" content_type="text"> Mahadevan, P., Wofsy, S. C., Matross, D. M., Xiao, X., Dunn, A. L., Lin, J. C., Gerbig, C., Munger, J. W., Chow, V. Y., and Gottlieb, E. W.: A satellite-based biosphere parameterization for net ecosystem CO2 exchange: Vegetation Photosynthesis and Respiration Model (VPRM), Global Biogeochem. Cy., 22, GB2005, doi:2010.1029/2006GB002735, 2008. </reference>
		<reference numeration="18" content_type="text"> Miller, C. E., Crisp, D., DeCola, P. L., Olsen, S. C., Randerson, J. T., Michalak, A. M., Alkhaled, A., Rayner, P., Jacob, D. J., Suntharalingam, P., Jones, D. B. A., Denning, A. S., Nicholls, M. E., Doney, S. C., Pawson, S., Boesch, H., Connor, B. J., Fung, I. Y., O&apos;Brien, D., Salawitch, R. J., Sander, S. P., Sen, B., Tans, P., Toon, G. C., Wennberg, P. O., Wofsy, S. C., Yung, Y. L., and Law, R. M.: Precision requirements for space-based XCO2 data, J. Geophys. Res., 112, D10314, doi:10.1029/2006JD007659, 2007. </reference>
		<reference numeration="19" content_type="text"> NIES: GOSAT: Greenhouse Gases Observing Satellite, Tsukuba, Japan, 2006. </reference>
		<reference numeration="20" content_type="text"> Parazoo, N. C., Denning, A. S., Kawa, S. R., Corbin, K. D., Lokupitiya, R. S., and Baker, I. T.: Mechanisms for synoptic variations of atmospheric CO&lt;sub&gt;2&lt;/sub&gt; in North America, South America and Europe, Atmos. Chem. Phys., 8, 7239–7254, 2008. </reference>
		<reference numeration="21" content_type="text"> Peters, W., Jacobson, A. R., Sweeney, C., Andrews, A. E., Conway, T. J., Masarie, K., Miller, J. B., Bruhwiler, L. M. P., P&apos; etron, G., Hirsch, A. I., Worthy, D. E. J., van der Werf, G. R., Randerson, J. T., Wennberg, P. O., Krol, M. C., and Tans, P. P.: An atmospheric perspective on North American carbon dioxide exchange: CarbonTracker, P. Natl. Acad. Sci. USA, 104, 18925–18930, 2007. </reference>
		<reference numeration="22" content_type="text"> Rayner, P. J. and O&apos;Brien, D. M.: The utility of remotely sensed CO2 concentration data in surface source inversions, Geophys. Res. Lett., 28, 175–178, 2001. </reference>
		<reference numeration="23" content_type="text"> Rödenbeck, C., Houweling, S., Gloor, M., and Heimann, M.: CO&lt;sub&gt;2&lt;/sub&gt; flux history 1982-2001 inferred from atmospheric data using a global inversion of atmospheric transport, Atmos. Chem. Phys., 3, 1919–1964, 2003. </reference>
		<reference numeration="24" content_type="text"> Takahashi, T., Sutherland, S. C., Sweeney, C., Poisson, A., Metzl, N., Tilbrook, B., Bates, N., Wanninkhof, R., Feely, R. A., Sabine, C., Olafsson, J., and Nojiri, Y.: Global sea-air CO2 flux based on climatological surface ocean $p$CO2, and seasonal biological and temperature effects, Deep-Sea Res. Pt. II, 49, 1601–1622, 2002. </reference>
		<reference numeration="25" content_type="text"> Tolk, L. F., Meesters, A. G. C. A., Dolman, A. J., and Peters, W.: Modelling representation errors of atmospheric CO&lt;sub&gt;2&lt;/sub&gt; mixing ratios at a regional scale, Atmos. Chem. Phys., 8, 6587–6596, 2008. </reference>
		<reference numeration="26" content_type="text"> van der Molen, M. K. and Dolman, A. J.: Regional carbon fluxes and the effect of topography on the variability of atmospheric CO2, J. Geophys. Res.-Atmos., 112, D01104, doi:01110.01029/02006JD007649, 2007. </reference>
	</references>
</article>

