ACP Atmospheric Chemistry and Physics ACP 1680-7324 Copernicus GmbH Göttingen, Germany 10.5194/acp-10-7017-2010 Historical (1850–2000) gridded anthropogenic and biomass burning emissions of reactive gases and aerosols: methodology and application Lamarque J.-F. 1 Bond T. C. 2 Eyring V. 3 Granier C. 4 5 6 Heil A. 7 Klimont Z. 8 Lee D. 9 Liousse C. 10 Mieville A. 6 Owen B. 9 Schultz M. G. 7 Shindell D. 11 Smith S. J. 12 Stehfest E. 13 Van Aardenne J. 14 Cooper O. R. 4 Kainuma M. 15 Mahowald N. 16 McConnell J. R. 17 Naik V. 18 Riahi K. 8 van Vuuren D. P. 13 National Center for Atmospheric Research, Boulder, USA University of Illinois, Urbana-Champaign, IL, USA Deutsches Zentrum fuer Luft- und Raumfahrt (DLR), Institut für Physik der Atmosphäre, Oberpfaffenhoffen, Germany NOAA Earth System Research Laboratory, Chemical Sciences Division, Boulder, CO, USA Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, Colorado, USA UPMC Univ. Paris 06; CNRS/INSU, UMR 8190 LATMOS-IPSL, Paris, France, France Forschungszentrum, Jülich, Germany International Institute for Applied Systems Analysis, Laxenburg, Austria Manchester Metropolitan University, Manchester, UK Laboratoire d'Aérologie, Toulouse, France Goddard Institute for Space Studies, National Aeronautics and Space Agency, New York, NY, USA Joint Global Change Research Institute, Pacific Northwest National Laboratory, College Park, MD, USA Netherlands Environmental Assessment Agency, Bilthoven, The Netherlands European Commission, DG, Joint Research Center, Ispra, Italy National Institute of Environmental Studies, Tsukuba, Japan Cornell University, Ithaca, New York, USA Desert Research Institute, Reno, Nevada, USA High Performance Technologies Inc./NOAA Geophysical Fluid Dynamics Laboratory, Princeton, NJ, USA 03 08 2010 10 15 7017 7039 This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited. This article is available from http://www.atmos-chem-phys.net/10/7017/2010/acp-10-7017-2010.html The full text article is available as a PDF file from http://www.atmos-chem-phys.net/10/7017/2010/acp-10-7017-2010.pdf

We present and discuss a new dataset of gridded emissions covering the historical period (1850–2000) in decadal increments at a horizontal resolution of 0.5° in latitude and longitude. The primary purpose of this inventory is to provide consistent gridded emissions of reactive gases and aerosols for use in chemistry model simulations needed by climate models for the Climate Model Intercomparison Program #5 (CMIP5) in support of the Intergovernmental Panel on Climate Change (IPCC) Fifth Assessment report (AR5). Our best estimate for the year 2000 inventory represents a combination of existing regional and global inventories to capture the best information available at this point; 40 regions and 12 sectors are used to combine the various sources. The historical reconstruction of each emitted compound, for each region and sector, is then forced to agree with our 2000 estimate, ensuring continuity between past and 2000 emissions. Simulations from two chemistry-climate models are used to test the ability of the emission dataset described here to capture long-term changes in atmospheric ozone, carbon monoxide and aerosol distributions. The simulated long-term change in the Northern mid-latitudes surface and mid-troposphere ozone is not quite as rapid as observed. However, stations outside this latitude band show much better agreement in both present-day and long-term trend. The model simulations indicate that the concentration of carbon monoxide is underestimated at the Mace Head station; however, the long-term trend over the limited observational period seems to be reasonably well captured. The simulated sulfate and black carbon deposition over Greenland is in very good agreement with the ice-core observations spanning the simulation period. Finally, aerosol optical depth and additional aerosol diagnostics are shown to be in good agreement with previously published estimates and observations.

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