<?xml version="1.0" encoding="UTF-8"?>
<!DOCTYPE article PUBLIC "-//NLM//DTD Journal Publishing DTD v3.0 20080202//EN" "http://dtd.nlm.nih.gov/publishing/3.0/journalpublishing3.dtd">
<article xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink" article-type="research-article" dtd-version="3.0" xml:lang="en">
<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACP</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7324</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>GÃ¶ttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acp-10-3107-2010</article-id>
<title-group>
<article-title>What can we learn from European continuous atmospheric CO&lt;sub&gt;2&lt;/sub&gt; measurements to quantify regional fluxes â€“ Part 1: Potential of the 2001 network</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Carouge</surname>
<given-names>C.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Bousquet</surname>
<given-names>P.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Peylin</surname>
<given-names>P.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Rayner</surname>
<given-names>P. J.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Ciais</surname>
<given-names>P.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Laboratoire des Sciences du Climat et de l&apos;Environnement, UMR1572 CNRS-CEA-UVSQ, BÃ¢t. 701, Orme des Merisiers, 91191 Gif-sur-Yvette, France</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>UniversitÃ© de Versailles Saint-Quentin en Yvelines, Versailles, France</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>Laboratoire de BiogÃ©ochimie et Ecologie des Milieux Continentaux, CNRS-UPMC-INRA, Paris, France</addr-line>
</aff>
<pub-date pub-type="epub">
<day>31</day>
<month>03</month>
<year>2010</year>
</pub-date>
<volume>10</volume>
<issue>6</issue>
<fpage>3107</fpage>
<lpage>3117</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
<self-uri xlink:href="http://www.atmos-chem-phys.net/10/3107/2010/acp-10-3107-2010.html">This article is available from http://www.atmos-chem-phys.net/10/3107/2010/acp-10-3107-2010.html</self-uri>
<self-uri xlink:href="http://www.atmos-chem-phys.net/10/3107/2010/acp-10-3107-2010.pdf">The full text article is available as a PDF file from http://www.atmos-chem-phys.net/10/3107/2010/acp-10-3107-2010.pdf</self-uri>
<abstract>
<p>An inverse model using atmospheric CO&lt;sub&gt;2&lt;/sub&gt; observations from a European
network of stations to reconstruct daily CO&lt;sub&gt;2&lt;/sub&gt; fluxes and their
uncertainties over Europe at 40 km resolution has been developed within a
Bayesian framework. In this first part, a pseudo-data experiment is
performed to assess the potential of continuous measurements over Europe
using a network of 10 stations of the AEROCARB project such as in 2001
(&lt;a href=&quot;http://www.aerocarb.cnrs-gif.fr/&quot;target=&quot;_blank&quot;&gt;http://www.aerocarb.cnrs-gif.fr/&lt;/a&gt;). Under the assumptions of a small
observation noise and a perfect atmospheric transport model, the
reconstruction of daily CO&lt;sub&gt;2&lt;/sub&gt; fluxes and in particular of their synoptic
variability is best over Western Europe where the network is the densest. At
least a 10 days temporal and a 1000 km spatial averaging of the inverted
daily/40 km fluxes is required in order to obtain a good agreement between
the estimated and the &quot;true&quot; fluxes in terms of correlation and
variability. The performance of the inversion system rapidly degrades when
fluxes are sought for a smaller temporal or spatial averaging.</p>
</abstract>
<counts><page-count count="11"/></counts>
</article-meta>
</front>
<body/>
<back>
<ref-list>
<title>References</title>
<ref id="ref1">
<label>1</label><mixed-citation publication-type="other" xlink:type="simple">Bousquet, P., Ciais, P., Miller, J. B., Dlugokencky, E. J., Hauglustaine, D. A., Prigent, C., van der Werf, G. R., Peylin, P., Brunke, E.-G., Carouge, C., Langenfelds, R. L., Lathiere, J., Papa, F., Ramonet, M., Schmidt, M., Steele, L. P., Tyler, S. C., and White, J.: Contribution of anthropogenic and natural sources to atmospheric methane variability, Nature, 443(7110), 439â€“443, 2006. </mixed-citation>
</ref>
<ref id="ref2">
<label>2</label><mixed-citation publication-type="other" xlink:type="simple">Bousquet, P., Hauglustaine, D. A., Peylin, P., Carouge, C., and Ciais, P.: Two decades of OH variability as inferred by an inversion of atmospheric transport and chemistry of methyl chloroform, Atmos. Chem. Phys., 5, 2635â€“2656, 2005. </mixed-citation>
</ref>
<ref id="ref3">
<label>3</label><mixed-citation publication-type="other" xlink:type="simple"> Carouge, C., Rayner, P. J., Peylin, P., Bousquet, P., Chevallier, F., and Ciais, P.: What can we learn from European continuous atmospheric CO&lt;sub&gt;2&lt;/sub&gt; measurements to quantify regional fluxes â€“ Part~2: Sensitivity of flux accuracy to inverse setup, Atmos. Chem. Phys., 10, 3119-3129, 2010. </mixed-citation>
</ref>
<ref id="ref4">
<label>4</label><mixed-citation publication-type="other" xlink:type="simple">Chevallier, F., Breon, F.-M., and Rayner, P. J.: Contribution of the Orbiting Carbon Observatory to the estimation of CO&lt;sub&gt;2&lt;/sub&gt; sources and sinks: Theoretical study in a variational data assimilation framework, J. Geophys. Res.-Atmos., 112(D9), D09307, doi:10.1029/2006JD007375, 2007. %</mixed-citation>
</ref>
<ref id="ref5">
<label>5</label><mixed-citation publication-type="other" xlink:type="simple">Carouge, C., Peylin, P., Rayner, P. J., Bousquet, P., Chevallier, F., and %Ciais, P.: What can we learn from European continuous atmospheric CO2 %measurements to quantify regional fluxes â€“ Part 2: Sensitivity of flux %accuracy to inverse setup, Atmos. Chem. Phys. Discuss., 8, 18621â€“18649, %2008. </mixed-citation>
</ref>
<ref id="ref6">
<label>6</label><mixed-citation publication-type="other" xlink:type="simple">Chevallier, F., Viovy, N., Reichstein, M., and Ciais, P.: On the assignment of prior errors in Bayesian inversions of CO&lt;sub&gt;2&lt;/sub&gt; surface fluxes, Geophys. Res. Lett., 33(13), L13802, doi:10.1029/2006GL026496, 2006. </mixed-citation>
</ref>
<ref id="ref7">
<label>7</label><mixed-citation publication-type="other" xlink:type="simple">Geels, C., Gloor, M., Ciais, P., Bousquet, P., Peylin, P., Vermeulen, A. T., Dargaville, R., Aalto, T., Brandt, J., Christensen, J. H., Frohn, L. M., Haszpra, L., Karstens, U., RÃ¶denbeck, C., Ramonet, M., Carboni, G., and Santaguida, R.: Comparing atmospheric transport models for future regional inversions over Europe – Part 1: mapping the atmospheric CO&lt;sub&gt;2&lt;/sub&gt; signals, Atmos. Chem. Phys., 7, 3461â€“3479, 2007. </mixed-citation>
</ref>
<ref id="ref8">
<label>8</label><mixed-citation publication-type="other" xlink:type="simple">Gerbig, C., Lin, J. C., Wofsy, S. C., Daube, B. C., Andrews, A. E., Stephens, B. B., Bakwin, P. S., amd Grainger, C. A.: Toward constraining regional-scale fluxes of CO&lt;sub&gt;2&lt;/sub&gt; with atmospheric observations over a continent: 1. Observed spatial variability from airborne platforms, J. Geophys. Res.-Atmos., 108(D24), 4756, doi:10.1029/2002JD003018, 2003. </mixed-citation>
</ref>
<ref id="ref9">
<label>9</label><mixed-citation publication-type="other" xlink:type="simple">Gloor, M., Fan, S. M., Pacala, S., and Sarmiento, J.: Optimal sampling of the atmosphere for purpose of inverse modeling: A model study, Global Biogeochem. Cy., 14(1), 407â€“428, 2000. </mixed-citation>
</ref>
<ref id="ref10">
<label>10</label><mixed-citation publication-type="other" xlink:type="simple">Gurney, K. R., Chen, Y. H., Maki, T., Kawa, S. R., Andrews, A., and Zhu, Z. X.: Sensitivity of atmospheric CO&lt;sub&gt;2&lt;/sub&gt; inversions to seasonal and interannual variations in fossil fuel emissions, J. Geophys. Res.-Atmos., 110(D10), D10308, doi:10.1029/2004JD005373, 2005. </mixed-citation>
</ref>
<ref id="ref11">
<label>11</label><mixed-citation publication-type="other" xlink:type="simple">Gurney, K.R., Law, R. M., Denning, A. S., Rayner, P. J., Baker, D., Bousquet, P., Bruhwiler, L., Chen, Y. H., Ciais, P., Fan, S., Fung, I. Y., Gloor, M., Heimann, M., Higuchi, K., John, J., Maki, T., Maksyutov, S., Masarie, K., Peylin, P., Prather, M., Pak, B. C., Randerson, J., Sarmiento, J., Taguchi, S., Takahashi, T., and Yuen, C. W.: Towards robust regional estimates of CO&lt;sub&gt;2&lt;/sub&gt; sources and sinks using atmospheric transport models, Nature, 415(6872), 626â€“630, 2002. </mixed-citation>
</ref>
<ref id="ref12">
<label>12</label><mixed-citation publication-type="other" xlink:type="simple">Hauglustaine, D. A., Hourdin, F., Jourdain, L., Filiberti, M.-A., Walters, S., Lamarque, J.-F., and Holland E. A.: Interactive chemistry in the Laboratoire de Météorologie Dynamique general circulation model: Description and background tropospheric chemistry evaluation, J. Geophys. Res., 109, D04314, doi:10.1029/2003JD003957, 2004. </mixed-citation>
</ref>
<ref id="ref13">
<label>13</label><mixed-citation publication-type="other" xlink:type="simple">Hourdin, F. and Talagrand, O.: Eulerian backtracking of atmospheric tracers: I Adjoint derivation and parametrization of subgrid-scale transport, Q. J. Roy. Meteor. Soc., 132(615), 567â€“583, 2006a. </mixed-citation>
</ref>
<ref id="ref14">
<label>14</label><mixed-citation publication-type="other" xlink:type="simple">Hourdin, F., Talagrand, O., and Idelkadi, A.: Eulerian backtracking of atmospheric tracers: II Numerical aspects, Q. J. Roy. Meteor. Soc., 132(615), 583â€“603, 2006b. </mixed-citation>
</ref>
<ref id="ref15">
<label>15</label><mixed-citation publication-type="other" xlink:type="simple">Hourdin, F. and Armengaud, A.: The use of finite-volume methods for atmospheric advection of trace species. Part I: Test of various formulations in a general circulation model, Mon. Weather Rev., 127(5), 822â€“837, 1999. </mixed-citation>
</ref>
<ref id="ref16">
<label>16</label><mixed-citation publication-type="other" xlink:type="simple"> IPCC, 2007: Climate Change 2007: The Physical Science Basis. Contribution of Working Group I to the Fourth Assessment Report of the Intergovernmental Panel on Climate Change, edited by: Solomon, S., Qin, D., Manning, M., Chen, Z., Marquis, M., Averyt, K. B., Tignor, M., and Miller, H. L., Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA, 996 pp., 2007. </mixed-citation>
</ref>
<ref id="ref17">
<label>17</label><mixed-citation publication-type="other" xlink:type="simple">Issartel, J.-P. and Baverel, J.: Inverse transport for the verification of the Comprehensive Nuclear Test Ban Treaty, Atmos. Chem. Phys., 3, 475â€“486, 2003. </mixed-citation>
</ref>
<ref id="ref18">
<label>18</label><mixed-citation publication-type="other" xlink:type="simple">Jung, M., Le Maire, G., Zaehle, S., Luyssaert, S., Vetter, M., Churkina, G., Ciais, P., Viovy, N., and Reichstein, M.: Assessing the ability of three land ecosystem models to simulate gross carbon uptake of forests from boreal to Mediterranean climate in Europe, Biogeosciences, 4, 647â€“656, 2007. </mixed-citation>
</ref>
<ref id="ref19">
<label>19</label><mixed-citation publication-type="other" xlink:type="simple">Kaminski, T., Rayner, P. J., Heimann, M., and Enting, I. G.: On aggregation errors in atmospheric transport inversions, J. Geophys. Res.-Atmos., 106(D5), 4703â€“4715, 2001. </mixed-citation>
</ref>
<ref id="ref20">
<label>20</label><mixed-citation publication-type="other" xlink:type="simple">Krinner, G., Viovy, N., de Noblet-Ducoudre, N., Ogee, J., Polcher, J., Friedlingstein, P., Ciais, P., Sitch, S., and Prentice, I. C.: A dynamic global vegetation model for studies of the coupled atmosphere-biosphere system, Global Biogeochem. Cy., 19(1), GB1015, doi:10.1029/2003GB002199, 2005. </mixed-citation>
</ref>
<ref id="ref21">
<label>21</label><mixed-citation publication-type="other" xlink:type="simple">Lafont, S., Kergoat, L., Dedieu, G., Chevillard, A., Karstens, U., and Kolle, O.: Spatial and temporal variability of land CO&lt;sub&gt;2&lt;/sub&gt; fluxes estimated with remote sensing and analysis data over western Eurasia., Tellus B, 54(5), 820â€“833, 2002. </mixed-citation>
</ref>
<ref id="ref22">
<label>22</label><mixed-citation publication-type="other" xlink:type="simple">Law, R. M., Rayner, P. J., Steele, L. P., and Enting, I. G.: Data and modelling requirements for CO&lt;sub&gt;2&lt;/sub&gt; inversions using high-frequency data, Tellus B, 55(2), 512â€“521, 2003. </mixed-citation>
</ref>
<ref id="ref23">
<label>23</label><mixed-citation publication-type="other" xlink:type="simple">Law, R. M., Rayner, P. J., Steele, L. P., and Enting, I. G.: Using high temporal frequency data for CO&lt;sub&gt;2&lt;/sub&gt; inversions, Global Biogeochem. Cy., 16(4), 1053, doi:10.1029/2001GB001593, 2002. </mixed-citation>
</ref>
<ref id="ref24">
<label>24</label><mixed-citation publication-type="other" xlink:type="simple">Peylin, P., Rayner, P. J., Bousquet, P., Carouge, C., Hourdin, F., Heinrich, P., Ciais, P., and AEROCARB contributors: Daily CO&lt;sub&gt;2&lt;/sub&gt; flux estimates over Europe from continuous atmospheric measurements: 1, inverse methodology, Atmos. Chem. Phys., 5, 3173â€“3186, 2005. </mixed-citation>
</ref>
<ref id="ref25">
<label>25</label><mixed-citation publication-type="other" xlink:type="simple">Rayner, P. J. and O&apos;Brien, D. M.: The utility of remotely sensed CO&lt;sub&gt;2&lt;/sub&gt; concentration data in surface source inversions, Geophys. Res. Lett., 28(1), 175â€“178, 2001. </mixed-citation>
</ref>
<ref id="ref26">
<label>26</label><mixed-citation publication-type="other" xlink:type="simple">RÃ¶denbeck, C., Houweling, S., Gloor, M., and Heimann, M.: CO&lt;sub&gt;2&lt;/sub&gt; flux history 1982â€“2001 inferred from atmospheric data using a global inversion of atmospheric transport, Atmos. Chem. Phys., 3, 1919â€“1964, 2003. </mixed-citation>
</ref>
<ref id="ref27">
<label>27</label><mixed-citation publication-type="other" xlink:type="simple">Sadourny, R. and Laval, K.: January and July performance of the LMD general circulation model, in: New perspectives in Climate Modeling, edited by: Berger, A. and Nicolis, C., 173â€“197, Elsevier, Amsterdam, 1984. </mixed-citation>
</ref>
<ref id="ref28">
<label>28</label><mixed-citation publication-type="other" xlink:type="simple">Saporta, G.: ProbabilitÃ©s, Analyse des donnÃ©es et Statistique, Technip, Paris, France, 1990. </mixed-citation>
</ref>
<ref id="ref29">
<label>29</label><mixed-citation publication-type="other" xlink:type="simple">Stephens, B. B., Gurney, K. R., Tans, P. P., Sweeney, C., Peters, W., Bruhwiler, L., Ciais, P., Rammonet, M., Bousquet, P., Nakazawa, T., Aoki, S., Machida, T., Inoue, G., Vinnichenko, N., Lloyd, J., Jordan, A., Shibistova, O., Lanenfelds, R. L., Stelle, L. P., Francey R. J., and Denning, A. S.: The vertical distribution of atmospheric CO&lt;sub&gt;2&lt;/sub&gt; defines the latitudinal partitioning of global carbon fluxes, Science, 316, 1732â€“1735, doi:10.1126/science.1137004, 2007. </mixed-citation>
</ref>
<ref id="ref30">
<label>30</label><mixed-citation publication-type="other" xlink:type="simple">Tarantola, A.: Inverse problem theory, Elsevier, Amsterdam, The Netherlands, 1987 </mixed-citation>
</ref>
<ref id="ref31">
<label>31</label><mixed-citation publication-type="other" xlink:type="simple">Thoning, K. W., Tans, P. P., and Komhyr, W. D.: Atmospheric carbon dioxide at Mauna Loa Observatory. 2. Analysis of the NOAA GMCC data, 1974, 1985, J. Geophys. Res.-Atmos., 94(D6), 8549â€“8565, 1989. </mixed-citation>
</ref>
<ref id="ref32">
<label>32</label><mixed-citation publication-type="other" xlink:type="simple">Tiedtke, M.: A comprehensive mass flux scheme for cumulus parametrization in large-scale models, Mon. Weather Rev., 117, 1179â€“1800, 1989. </mixed-citation>
</ref>
<ref id="ref33">
<label>33</label><mixed-citation publication-type="other" xlink:type="simple">Uppala, S. M., Kallberg, P. W., Simmons, A. J., Andrae, U., Bechtold, V. D., Fiorino, M., Gibson, J. K., Haseler, J., Hernandez, A., Kelly, G. A., Li, X., Onogi, K., Saarinen, S., Sokka, N., Allan, R. P., Andersson, E., Arpe, K., Balmaseda, M. A., Beljaars, A. C. M., Van De Berg, L., Bidlot, J., Bormann, N., Caires, S., Chevallier, F., Dethof, S., Dragosavac, M., Fisher, M., Fuentes, M., Hagemann, S., Holm, E., Hoskins, B. J., Isaksen, L., Janssen, P. A. E. M., Jenne, R., McNally, A. P., Mahfouf, J .F., Morcrette, J. J., Rayner, N. A., Saunders, R. W., Simon, P., Sterl, A., Trenberth, K. E., Untch, A., Vasiljevic, D., Viterbo, P., and Woollen, J.: The ERA-40 re-analysis, Q. J. Roy. Meteor. Soc., 131(612), 2961â€“3012, 2005. </mixed-citation>
</ref>
<ref id="ref34">
<label>34</label><mixed-citation publication-type="other" xlink:type="simple">Van Aardenne, J. A., Dentener, F. J., Olivier, J. G. J., Peters, J. A. H. W., and Ganzeveld, L. N.: The EDGAR 3.2 Fast Track 2000 dataset (32FT2000) â€“ Description of 32FT2000 (v.8).doc, http://www.mnp.nl/edgar/model/v32ft2000edgar/docv32ft2000/index.jsp, 2005. </mixed-citation>
</ref>
<ref id="ref35">
<label>35</label><mixed-citation publication-type="other" xlink:type="simple">Van Leer, B.: Towards the ultimate conservative difference scheme: IV. A new approach to numerical convection, J. Comput. Phys., 23, 276â€“299, 1977. </mixed-citation>
</ref>
</ref-list>
</back>
</article>